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gasherd: yes and no. It all depends on the type of material you're going for. Sometimes inverting the hue has a great effect because it negates color on highlights. Other materials may want no color, higher saturation same color, a small hue shift or light desaturation.
It's one of those questions where the final answer is: Depends. Experiment with materials, and test in game to see what looks the best. There's been a lot of questions about this around here lately, so I'll try and put together some information about speculars soon.
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